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For all three alkanes, the experimental and simulated nucleation rates are offset by âˆ❃ orders of magnitude when plotted as a function of ln S/(T c /T - 1) 1.5. Complementary Monte Carlo simulations, using the transferable potentials for phase equilibria-united atom potentials, suggest that despite the high degree of supercooling, the critical clusters remain liquid like under experimental conditions for n- pentane through n- heptane, but adopt more ordered structures for n-octane and n-nonane. For n- pentane and n- hexane, these are the first nucleation rate measurements that have been made, and the trends in the current data agree well with those in the earlier work of Ghosh et al. ![]() We measured the nucleation rates of n- pentane through n- heptane in a supersonic nozzle at temperatures ranging from ca. Ogunronbi, Kehinde E Sepehri, Aliasghar Chen, Bin Wyslouzil, Barbara E Vapor phase nucleation of the short-chain n-alkanes (n- pentane, n- hexane and n- heptane): Experiments and Monte Carlo simulations.
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